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Metamaterials have offered unprecedented potentials for wave manipulations. However, their applications in underwater acoustic wave control have remained largely unexplored. This is because of the limited material choices and the lack of reliable fabrication techniques for the complicated structures. Herein, a metamaterial with microlattice structures as the building blocks is proposed for underwater operations. By designing the building blocks of the metamaterial and assembling them in a layered fashion, anisotropy is embedded in the structure, which results along different effective sound speeds in orthogonal directions. The designed metamaterial is fabricated by metal additive manufacturing using aluminum and steel. Experiments are performed using a resonator tube to evaluate its performance in water. An anisotropy ratio of around 2 is achieved, which is in good agreement with numerical simulations. The proposed metamaterial provides an effective means for underwater sound control with reduced fabrication difficulties and increased service life. 

Abstract Acoustic metamaterials with negative constitutive parameters (modulus and/or mass density) have shown great potential in diverse applications ranging from sonic cloaking, abnormal refraction and superlensing, to noise canceling. In conventional acoustic metamaterials, the negative constitutive parameters are engineered via tailored structures with fixed geometries; therefore, the relationships between constitutive parameters and acoustic frequencies are typically fixed to form a 2D phase space once the structures are fabricated. Here, by means of a model system of magnetoactive lattice structures, stimuli‐responsive acoustic metamaterials are demonstrated to be able to extend the 2D phase space to 3D through rapidly and repeatedly switching signs of constitutive parameters with remote magnetic fields. It is shown for the first time that effective modulus can be reversibly switched between positive and negative within controlled frequency regimes through lattice buckling modulated by theoretically predicted magnetic fields. The magnetically triggered negative‐modulus and cavity‐induced negative density are integrated to achieve flexible switching between single‐negative and double‐negative. This strategy opens promising avenues for remote, rapid, and reversible modulation of acoustic transportation, refraction, imaging, and focusing in subwavelength regimes.